Title page for etd-0904109-195554


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URN etd-0904109-195554
Author Wei-Min Chin
Author's Email Address m963030013@student.nsysu.edu.tw
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Department Environmental Engineering
Year 2008
Semester 2
Degree Master
Type of Document
Language zh-TW.Big5 Chinese
Title Isotopic Characteristics of Asian Dusts and Their Physicochemical Succession of Long-Range Transport
Date of Defense 2009-06-05
Page Count 204
Keyword
  • Asian Continental Sandstorm (ACS)
  • Isotopic Properties
  • Source Regions
  • Physicochemical Characteristics Succession
  • Backward Trajectory
  • DMR Test
  • Abstract ABSTRACT
    In this study, we conducted an intensive sampling of Asian dusts at Pescadores Islands for heavy Asian continental sandstorms (ACS) from February 22 to March 6, 2008. To investigate the succession of anthropogenic and natural pollutants for the ACS transportation, PM2.5 and PM2.5-10 were sampled by two dichotomous samplers once every four hours during the ACS periods, and furthermore analyzed their physicochemical properties, including mass concentrations, particle size distribution, water-soluble ionic species, carbonaceous contents, and metallic contents. Experimental results indicated that it was mainly fine particles (PM2.5) prior to the ACS, and the percentage of anthropogenic species (i.e., SO42-, NH4+, NO3-, Zn, Mn and OC) increased dramatically. However, it changed to coarse particles while the ACS overwhelming, and the percentage of crustal/marine species (i.e., Cl-, Na+, Ca2+, Mg2+, Ca, Al, Mg and EC) increased. After the ACS, the concentrations of all species decreased substantially. However, the percentage of Cl- and Na+ increased, suggesting that sea breeze has constant influences on local suspended particles.
    In addition to the analysis of physicochemical properties of Asian dusts, this study applied a HYSPLIT MODEL to figure out the transportation routes and the source regions of the ACS. Backward trajectory analysis showed that the ACS was originated from the east portion of Inner Mongolia, namely the Onqin Daga Sandy Land and the Horqin Sandy Land. 
    Moreover, seventeen soil samples were collected from the Tengger Desert, the Mu Us Desert, the Onqin Daga Sandy Land, and the Horqin Sandy Land in Inner Mongolia during the year of 2005. The soil samples were resuspended in a resuspension chamber and then collected by a dichotomous sampler. This study focused on PM2.5-10 particles that mainly influence the downwind regions, and then took the ACS samples and the resuspended soil samples to measure the Sr isotopic characteristics of 87Sr/86Sr ratios by a multiple-collector inductively coupled plasma mass spectrometry (MC-ICP-MS). To characterize the isotopic properties of resuspended dust particles from the ACS source regions in northern China, and to correlate Asian dusts at the downwind regions of ACS with the source regions by Duncan’s Multiple Range Test (DMR). The DMR results showed that the ACS was probably originated from the east portion of Inner Mongolia, namely the Onqin Daga Sandy Land and the Horqin Sandy Land, which concurred with the backward trajectory analysis.
    Advisory Committee
  • Shui-Jen Chen - chair
  • Charles C.-K. Chou - co-chair
  • Chung-Hsuang Hung - co-chair
  • Chung-Shin Yuan - advisor
  • Files
  • etd-0904109-195554.pdf
  • indicate accessible in a year
    Date of Submission 2009-09-04

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